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Self-Powered Photodetector Fabricated from a Single-Charge-Transfer Complex Nanowire Grown In Situ between Prefabricated Electrodes on an Si3N4 Membrane

IR@CGCRI: CSIR-Central Glass and Ceramic Research Institute, Kolkata

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Title Self-Powered Photodetector Fabricated from a Single-Charge-Transfer Complex Nanowire Grown In Situ between Prefabricated Electrodes on an Si3N4 Membrane
 
Creator Basori, Rabaya
Raychaudhuri, Arup Kumar
 
Subject Electronics
 
Description Power consumption in an electronic circuit is one ofthe seriouschallenges that need to be improved to achieve a durable future. Aphotodetector is one such electronic device that consumes a huge externalpower to operate. This motivated the researchers to concentrate onself-powered optical photodetectors that can operate without externalbias. On the contrary, building a device on a transparent film ornanomembrane has great importance in the field of electronic skins,and lightweight and intelligent wearables technology. Here, we havereported the fabrication and characterization of a self-power opticalphotodetector device based on a single Cu:7,7,8,8-tetracyanoquinodimethanenanowire (Cu:TCNQ NW) of length & SIM;500 nm and diameter & SIM;50nm. The NW photodetector device was fabricated on a silicon nitride(Si3N4) membrane window (size = 100 & mu;mx 100 & mu;m, membrane thickness & SIM;100 nm) to meet thedemands of a lightweight and transparent technology. The reportedself-powered single-NW photodetector exhibits excellent photoresponsivity(& SIM;5.5 A/W), high detectivity (& SIM; 7 x 10(7) Jones), outstanding external quantum efficiency (& SIM;1.6 x10(3)%), and a large on/off current ratio (& SIM;1.5 x10(2)) at 49 nW optical power. The analysis reveals thatthe contribution is due to photocarrier generation, radial built-in-fieldon the NW's surface, and barrier height reduction during illumination.Self-powered optical photodetectors, in particular, have enormouspotential as novel emerging self-driven optoelectronic devices.
 
Publisher ACS Publications
 
Date 2023-06
 
Type Article
PeerReviewed
 
Identifier Basori, Rabaya and Raychaudhuri, Arup Kumar (2023) Self-Powered Photodetector Fabricated from a Single-Charge-Transfer Complex Nanowire Grown In Situ between Prefabricated Electrodes on an Si3N4 Membrane. ACS Applied Nano Materials, 6 (13). pp. 12560-12566. ISSN 2574-0970
 
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